Time-resolved measurement of interatomic coulombic decay in Ne2.

نویسندگان

  • K Schnorr
  • A Senftleben
  • M Kurka
  • A Rudenko
  • L Foucar
  • G Schmid
  • A Broska
  • T Pfeifer
  • K Meyer
  • D Anielski
  • R Boll
  • D Rolles
  • M Kübel
  • M F Kling
  • Y H Jiang
  • S Mondal
  • T Tachibana
  • K Ueda
  • T Marchenko
  • M Simon
  • G Brenner
  • R Treusch
  • S Scheit
  • V Averbukh
  • J Ullrich
  • C D Schröter
  • R Moshammer
چکیده

The lifetime of interatomic Coulombic decay (ICD) [L. S. Cederbaum et al., Phys. Rev. Lett. 79, 4778 (1997)] in Ne2 is determined via an extreme ultraviolet pump-probe experiment at the Free-Electron Laser in Hamburg. The pump pulse creates a 2s inner-shell vacancy in one of the two Ne atoms, whereupon the ionized dimer undergoes ICD resulting in a repulsive Ne+(2p(-1))-Ne+(2p(-1)) state, which is probed with a second pulse, removing a further electron. The yield of coincident Ne+-Ne2+ pairs is recorded as a function of the pump-probe delay, allowing us to deduce the ICD lifetime of the Ne2(+)(2s(-1)) state to be (150±50)  fs, in agreement with quantum calculations.

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عنوان ژورنال:
  • Physical review letters

دوره 111 9  شماره 

صفحات  -

تاریخ انتشار 2013